W0166
Impure Thoughts in Space (Dimer Impurities in Microgravity
Grown Lysozyme). Edward H. Snell, Russell A. Judge, Elizabeth L. Forsythe,
Marc L. Pusey, Michael Sportiello, Paul Todd, Henry Bellamy, Jeff Lovelace, John
M. Cassanto & Gloria E. O. Borgstahl, NASA Lab. for Structural Biology, Code
SD 48, NASA MSFC, Huntsville, AL 35812.
Chicken egg-white lysozyme (CEWL) crystals were grown in
microgravity and on the ground in the presence of various amounts of a naturally
occurring lysozyme dimer impurity. No significant favorable differences in
impurity incorporation between microgravity and ground crystal samples were
observed. At low impurity concentration the microgravity crystals preferentially
incorporated the dimer. The presence of the dimer in the crystallization
solutions in microgravity reduced crystal size, increased mosaicity and reduced
the signal to noise ratio of the X-ray data. Microgravity samples proved more
sensitive to impurity. Crystal quality was evaluated, in part, by measurement
of the angular width of hundreds of indexed reflections from each crystal. From
this data we were able to calculate the anisotropic mosaicity of each. The
largest crystals with the best X-ray diffraction properties were grown from pure
solution in microgravity. Microgravity should not be seen as a step to replace
good biochemical practice but may be useful in situations where solution
impurities are formed during the crystallization process. Partitioning of
impurities seems to be a complex phenomenon.