W0124
Molecular Approaches to Drug Design. Judith L.
Flippen-Anderson, Jeffrey R. Deschamps, and Clifford George, Laboratory for the
Structure of Matter, Code 6030, Naval Research Laboratory, Washington, DC
20375.
The history of opium predates the written word. Nicotine, the
most addictive drug available without prescription, is estimated to have
contributed to the loss of 400,000 lives in the United States alone in 1988.
More recent surveys indicate that there are nearly 400,000 people in the US
using cocaine on a daily basis with 5,000 new users being added every day. The
number of heroin users was estimated at more than 900,000 in 1999 with alarming
increases in usage by suburban teens. Billions of dollars are spent every year
in the "war" against these drugs. Ironically, many of these controlled
substances can provide release from intense pain. Control of these drugs lies
in being able to modify their properties, removing those that cause addiction
while retaining, or even improving, those properties that provide analgesia. To
do this we must understand their chemistry and biological activity. The key to
this understanding is hidden in the structures of these compounds, the ligands,
and in the structures of their receptors. If we can relate elements of
structure to chemical and biological properties we can begin to design new
compounds that can be used to treat drug abuse and to provide nearly complete
pain relief without addiction. The three-dimensional information provided by
x-ray crystallography, combined with computational methods can greatly enhance
the discovery of new compounds and can efficiently optimize their properties.
This presentation will focus on the x-ray structures of non-peptide ligands with
the aim of relating structure to function.